If you can't copy files that are bigger than 2 or 4 GB, usually HD movies and such, on to your USB key, it's usually due to the file system the USB key is formatted to.
In case you didn't know, you can turn you LG G2 Android powered smartphone into a Wi-Fi hotspot and use it to surf the web with any other wireless device like notebook, tablet or a smartphone.
If you are more of a visual person and would like to organize your folders and files using different colors, than check it out how to use color labels in Mac OS X.