1.
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Open a picture you want to make sharper in Gimp.
Yes, it's Kate Upton ;)
Click here for the how to add a High Pass Filter to Gimp tutorial.
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2.
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Go to layers window, and click Create a duplicate layer...
If you dont't see the layers press Ctrl + L to make it visible.
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3.
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In the menu click Filters, Generic and choose High Filter Pass ...
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4.
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... set Filter Radius and Contrast Adjust similar to my settings and click OK.
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5.
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Set the duplicated layer Mode to Overlay.
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